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FLOATSUBSCRIPTCl under 115 Ok. Its Br-containing analogue is stable within the room-temperature crystal structure right down to no less than 10 Okay, although the Br compound is on the verge of an analogous antiferroelectric instability and reveals native displacements of Cu and Br atoms. The I-containing compound is stable in its room-temperature construction in response to density-useful calculations. These parameters are chosen in a semi-empirical manner as providing best settlement with the experimental trade couplings in earlier DFT calculations for francisites Rousochatzakis et al. Quick-range AFM order is formed around 50 Okay, however no signatures of lengthy-vary ordering are seen down to 2 Okay. This conduct will be rationalized on the microscopic level by the spin lattice comprising sturdy non-pissed off one-dimensional (1D) units with solely weak and annoyed couplings between them. FLOATSUBSCRIPTCl, however its magnetic behavior is remarkably different. This habits is rationalized microscopically by way of a non-frustrated 1D spin ladder (tube) with comparatively weak and frustrated couplings between the 1D models. ARG antiferromagnets might be orders of magnitude decrease than the vitality scale of alternate couplings Janson et al. FLOATSUBSCRIPT tetrahedra. Most of the alternate couplings happen between nearest neighbors, however dissimilar interactions on the edges of those tetrahedra largely cut back the frustration and render the spin lattice quasi-1D.

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